Unconventional quantum oscillations and evidence of nonparabolic electronic states in quasi-two-dimensional electron system at complex oxide interfaces

The simultaneous occurrence of electric-field controlled superconductivity and spin-orbit interaction makes two-dimensional electron systems (2DES) constructed from perovskite transition metal oxides promising candidates for the next generation of spintronics and quantum computing. It is, however, e...

Full description

Saved in:
Bibliographic Details
Main Authors: Km Rubi, Denis R. Candido, Manish Dumen, Shengwei Zeng, Emily L.Q.N. Ammerlaan, Femke Bangma, Mun K. Chan, Michel Goiran, Ariando Ariando, Suvankar Chakraverty, Walter Escoffier, Uli Zeitler, Neil Harrison
Format: Article
Language:English
Published: American Physical Society 2024-12-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.6.043231
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1825208830968987648
author Km Rubi
Denis R. Candido
Manish Dumen
Shengwei Zeng
Emily L.Q.N. Ammerlaan
Femke Bangma
Mun K. Chan
Michel Goiran
Ariando Ariando
Suvankar Chakraverty
Walter Escoffier
Uli Zeitler
Neil Harrison
author_facet Km Rubi
Denis R. Candido
Manish Dumen
Shengwei Zeng
Emily L.Q.N. Ammerlaan
Femke Bangma
Mun K. Chan
Michel Goiran
Ariando Ariando
Suvankar Chakraverty
Walter Escoffier
Uli Zeitler
Neil Harrison
author_sort Km Rubi
collection DOAJ
description The simultaneous occurrence of electric-field controlled superconductivity and spin-orbit interaction makes two-dimensional electron systems (2DES) constructed from perovskite transition metal oxides promising candidates for the next generation of spintronics and quantum computing. It is, however, essential to understand the electronic bands thoroughly and verify the predicted electronic states experimentally in these 2DES to advance technological applications. Here, we present insights into the electronic states of the 2DES at oxide interfaces through comprehensive investigations of Shubnikov–de Haas oscillations in three different systems: EuO/KTaO_{3}, LaAlO_{3}/SrTiO_{3}, and amorphous-LaAlO_{3}/KTaO_{3}. To accurately resolve these oscillations, we conducted transport measurements in high magnetic fields up to 60 T and low temperatures down to 100 mK. For 2D confined electrons at these interfaces, we observed a progressive increase of oscillations frequency and cyclotron mass with the magnetic field. We interpret these universal and intriguing findings by considering the existence of nontrivial electronic bands, for which the E−k dispersion incorporates both linear and parabolic relations. In addition to providing experimental evidence for nonparabolic electronic states in KTaO_{3} and SrTiO_{3} 2DES, the unconventional oscillations presented in this study establish a paradigm for quantum oscillations in 2DES based on perovskite transition metal oxides, where the oscillation frequencies in 1/B exhibit quadratic dependence on the magnetic field.
format Article
id doaj-art-063aa92fbe204fed88dc786b88f4d7e2
institution Kabale University
issn 2643-1564
language English
publishDate 2024-12-01
publisher American Physical Society
record_format Article
series Physical Review Research
spelling doaj-art-063aa92fbe204fed88dc786b88f4d7e22025-02-06T17:04:09ZengAmerican Physical SocietyPhysical Review Research2643-15642024-12-016404323110.1103/PhysRevResearch.6.043231Unconventional quantum oscillations and evidence of nonparabolic electronic states in quasi-two-dimensional electron system at complex oxide interfacesKm RubiDenis R. CandidoManish DumenShengwei ZengEmily L.Q.N. AmmerlaanFemke BangmaMun K. ChanMichel GoiranAriando AriandoSuvankar ChakravertyWalter EscoffierUli ZeitlerNeil HarrisonThe simultaneous occurrence of electric-field controlled superconductivity and spin-orbit interaction makes two-dimensional electron systems (2DES) constructed from perovskite transition metal oxides promising candidates for the next generation of spintronics and quantum computing. It is, however, essential to understand the electronic bands thoroughly and verify the predicted electronic states experimentally in these 2DES to advance technological applications. Here, we present insights into the electronic states of the 2DES at oxide interfaces through comprehensive investigations of Shubnikov–de Haas oscillations in three different systems: EuO/KTaO_{3}, LaAlO_{3}/SrTiO_{3}, and amorphous-LaAlO_{3}/KTaO_{3}. To accurately resolve these oscillations, we conducted transport measurements in high magnetic fields up to 60 T and low temperatures down to 100 mK. For 2D confined electrons at these interfaces, we observed a progressive increase of oscillations frequency and cyclotron mass with the magnetic field. We interpret these universal and intriguing findings by considering the existence of nontrivial electronic bands, for which the E−k dispersion incorporates both linear and parabolic relations. In addition to providing experimental evidence for nonparabolic electronic states in KTaO_{3} and SrTiO_{3} 2DES, the unconventional oscillations presented in this study establish a paradigm for quantum oscillations in 2DES based on perovskite transition metal oxides, where the oscillation frequencies in 1/B exhibit quadratic dependence on the magnetic field.http://doi.org/10.1103/PhysRevResearch.6.043231
spellingShingle Km Rubi
Denis R. Candido
Manish Dumen
Shengwei Zeng
Emily L.Q.N. Ammerlaan
Femke Bangma
Mun K. Chan
Michel Goiran
Ariando Ariando
Suvankar Chakraverty
Walter Escoffier
Uli Zeitler
Neil Harrison
Unconventional quantum oscillations and evidence of nonparabolic electronic states in quasi-two-dimensional electron system at complex oxide interfaces
Physical Review Research
title Unconventional quantum oscillations and evidence of nonparabolic electronic states in quasi-two-dimensional electron system at complex oxide interfaces
title_full Unconventional quantum oscillations and evidence of nonparabolic electronic states in quasi-two-dimensional electron system at complex oxide interfaces
title_fullStr Unconventional quantum oscillations and evidence of nonparabolic electronic states in quasi-two-dimensional electron system at complex oxide interfaces
title_full_unstemmed Unconventional quantum oscillations and evidence of nonparabolic electronic states in quasi-two-dimensional electron system at complex oxide interfaces
title_short Unconventional quantum oscillations and evidence of nonparabolic electronic states in quasi-two-dimensional electron system at complex oxide interfaces
title_sort unconventional quantum oscillations and evidence of nonparabolic electronic states in quasi two dimensional electron system at complex oxide interfaces
url http://doi.org/10.1103/PhysRevResearch.6.043231
work_keys_str_mv AT kmrubi unconventionalquantumoscillationsandevidenceofnonparabolicelectronicstatesinquasitwodimensionalelectronsystematcomplexoxideinterfaces
AT denisrcandido unconventionalquantumoscillationsandevidenceofnonparabolicelectronicstatesinquasitwodimensionalelectronsystematcomplexoxideinterfaces
AT manishdumen unconventionalquantumoscillationsandevidenceofnonparabolicelectronicstatesinquasitwodimensionalelectronsystematcomplexoxideinterfaces
AT shengweizeng unconventionalquantumoscillationsandevidenceofnonparabolicelectronicstatesinquasitwodimensionalelectronsystematcomplexoxideinterfaces
AT emilylqnammerlaan unconventionalquantumoscillationsandevidenceofnonparabolicelectronicstatesinquasitwodimensionalelectronsystematcomplexoxideinterfaces
AT femkebangma unconventionalquantumoscillationsandevidenceofnonparabolicelectronicstatesinquasitwodimensionalelectronsystematcomplexoxideinterfaces
AT munkchan unconventionalquantumoscillationsandevidenceofnonparabolicelectronicstatesinquasitwodimensionalelectronsystematcomplexoxideinterfaces
AT michelgoiran unconventionalquantumoscillationsandevidenceofnonparabolicelectronicstatesinquasitwodimensionalelectronsystematcomplexoxideinterfaces
AT ariandoariando unconventionalquantumoscillationsandevidenceofnonparabolicelectronicstatesinquasitwodimensionalelectronsystematcomplexoxideinterfaces
AT suvankarchakraverty unconventionalquantumoscillationsandevidenceofnonparabolicelectronicstatesinquasitwodimensionalelectronsystematcomplexoxideinterfaces
AT walterescoffier unconventionalquantumoscillationsandevidenceofnonparabolicelectronicstatesinquasitwodimensionalelectronsystematcomplexoxideinterfaces
AT ulizeitler unconventionalquantumoscillationsandevidenceofnonparabolicelectronicstatesinquasitwodimensionalelectronsystematcomplexoxideinterfaces
AT neilharrison unconventionalquantumoscillationsandevidenceofnonparabolicelectronicstatesinquasitwodimensionalelectronsystematcomplexoxideinterfaces