Recent advancements in durable and self-healing oil well cement: A pathway to secure carbon sequestration

Carbon capture, utilization, and storage (CCUS) technology plays a critical role for significantly reducing greenhouse gas emissions. The integrity of the cement sheath in storage wells is essential to secure the subsurface CO2 storage, however, acidic CO2 can erode the cement sheath over time, lead...

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Main Authors: Yan Xie, Michelle Tiong, Qi Liu, Tong Wu, Wanzhen Xue, Chunkai Wang
Format: Article
Language:English
Published: Elsevier 2025-02-01
Series:Journal of CO2 Utilization
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2212982025000204
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author Yan Xie
Michelle Tiong
Qi Liu
Tong Wu
Wanzhen Xue
Chunkai Wang
author_facet Yan Xie
Michelle Tiong
Qi Liu
Tong Wu
Wanzhen Xue
Chunkai Wang
author_sort Yan Xie
collection DOAJ
description Carbon capture, utilization, and storage (CCUS) technology plays a critical role for significantly reducing greenhouse gas emissions. The integrity of the cement sheath in storage wells is essential to secure the subsurface CO2 storage, however, acidic CO2 can erode the cement sheath over time, leading to chemical and mechanical damages of cement, risking CO2 leakage. The advancement of nanotechnology has introduced nanomaterials into cementing operations, enhancing oil well cement durability against storage conditions due to their high surface area and reactivity. To enhance the security of CO2 storage, it is proposed to incorporate self-healing materials into the cement, which autonomously repair microcracks to maintain the cement sheath's sealing integrity. This review firstly discusses the hydration and carbonation processes of in wellbore cement, and evaluates the influences of various nanomaterials on the cement durability. Subsequently, the self-healing mechanisms of such cement is introduced, along with the effects of different materials on the self-healing performance of oil well cement. Finally, by analyzing existing research achievements and issues, the future important research directions are provided.
format Article
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institution Kabale University
issn 2212-9839
language English
publishDate 2025-02-01
publisher Elsevier
record_format Article
series Journal of CO2 Utilization
spelling doaj-art-297384d5951e46e49003b727dc1b67cb2025-02-08T05:00:22ZengElsevierJournal of CO2 Utilization2212-98392025-02-0192103036Recent advancements in durable and self-healing oil well cement: A pathway to secure carbon sequestrationYan Xie0Michelle Tiong1Qi Liu2Tong Wu3Wanzhen Xue4Chunkai Wang5National Key Laboratory of Petroleum Resources and Engineering, Unconventional Petroleum Research Institute, China University of Petroleum, Beijing, Beijing 102249, ChinaCorresponding authors.; National Key Laboratory of Petroleum Resources and Engineering, Unconventional Petroleum Research Institute, China University of Petroleum, Beijing, Beijing 102249, ChinaCorresponding authors.; National Key Laboratory of Petroleum Resources and Engineering, Unconventional Petroleum Research Institute, China University of Petroleum, Beijing, Beijing 102249, ChinaNational Key Laboratory of Petroleum Resources and Engineering, Unconventional Petroleum Research Institute, China University of Petroleum, Beijing, Beijing 102249, ChinaNational Key Laboratory of Petroleum Resources and Engineering, Unconventional Petroleum Research Institute, China University of Petroleum, Beijing, Beijing 102249, ChinaNational Key Laboratory of Petroleum Resources and Engineering, Unconventional Petroleum Research Institute, China University of Petroleum, Beijing, Beijing 102249, ChinaCarbon capture, utilization, and storage (CCUS) technology plays a critical role for significantly reducing greenhouse gas emissions. The integrity of the cement sheath in storage wells is essential to secure the subsurface CO2 storage, however, acidic CO2 can erode the cement sheath over time, leading to chemical and mechanical damages of cement, risking CO2 leakage. The advancement of nanotechnology has introduced nanomaterials into cementing operations, enhancing oil well cement durability against storage conditions due to their high surface area and reactivity. To enhance the security of CO2 storage, it is proposed to incorporate self-healing materials into the cement, which autonomously repair microcracks to maintain the cement sheath's sealing integrity. This review firstly discusses the hydration and carbonation processes of in wellbore cement, and evaluates the influences of various nanomaterials on the cement durability. Subsequently, the self-healing mechanisms of such cement is introduced, along with the effects of different materials on the self-healing performance of oil well cement. Finally, by analyzing existing research achievements and issues, the future important research directions are provided.http://www.sciencedirect.com/science/article/pii/S2212982025000204CCUSOil well cementCO2 corrosionNanomaterialsSelf-healing
spellingShingle Yan Xie
Michelle Tiong
Qi Liu
Tong Wu
Wanzhen Xue
Chunkai Wang
Recent advancements in durable and self-healing oil well cement: A pathway to secure carbon sequestration
Journal of CO2 Utilization
CCUS
Oil well cement
CO2 corrosion
Nanomaterials
Self-healing
title Recent advancements in durable and self-healing oil well cement: A pathway to secure carbon sequestration
title_full Recent advancements in durable and self-healing oil well cement: A pathway to secure carbon sequestration
title_fullStr Recent advancements in durable and self-healing oil well cement: A pathway to secure carbon sequestration
title_full_unstemmed Recent advancements in durable and self-healing oil well cement: A pathway to secure carbon sequestration
title_short Recent advancements in durable and self-healing oil well cement: A pathway to secure carbon sequestration
title_sort recent advancements in durable and self healing oil well cement a pathway to secure carbon sequestration
topic CCUS
Oil well cement
CO2 corrosion
Nanomaterials
Self-healing
url http://www.sciencedirect.com/science/article/pii/S2212982025000204
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AT qiliu recentadvancementsindurableandselfhealingoilwellcementapathwaytosecurecarbonsequestration
AT tongwu recentadvancementsindurableandselfhealingoilwellcementapathwaytosecurecarbonsequestration
AT wanzhenxue recentadvancementsindurableandselfhealingoilwellcementapathwaytosecurecarbonsequestration
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