Impact of the COVID-19 Event on the Characteristics of Atmospheric Single Particle in the Northern China

Abstract The COVID-19 event triggered global attention which broke out at the end of 2019. To investigate the impact of the COVID-19 pandemic prevention and control actions on the chemical composition, size distribution, and mixing state of individual particles, real-time individual particles in the...

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Main Authors: Zheng Li, Jingjing Meng, Ling Zhou, Ruiwen Zhou, Mengxuan Fu, Yachen Wang, Yanan Yi, Aijing Song, Qingchun Guo, Zhanfang Hou, Li Yan
Format: Article
Language:English
Published: Springer 2024-12-01
Series:Aerosol and Air Quality Research
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Online Access:https://doi.org/10.4209/aaqr.2020.06.0321
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author Zheng Li
Jingjing Meng
Ling Zhou
Ruiwen Zhou
Mengxuan Fu
Yachen Wang
Yanan Yi
Aijing Song
Qingchun Guo
Zhanfang Hou
Li Yan
author_facet Zheng Li
Jingjing Meng
Ling Zhou
Ruiwen Zhou
Mengxuan Fu
Yachen Wang
Yanan Yi
Aijing Song
Qingchun Guo
Zhanfang Hou
Li Yan
author_sort Zheng Li
collection DOAJ
description Abstract The COVID-19 event triggered global attention which broke out at the end of 2019. To investigate the impact of the COVID-19 pandemic prevention and control actions on the chemical composition, size distribution, and mixing state of individual particles, real-time individual particles in the urban atmosphere of the Northern China were analyzed using single particle aerosol mass spectrometry (SPAMS) during January 16 to February 4, 2020. The results showed that the concentrations of PM2.5, NOx, and CO were lower during DP (during the pandemic) than those during BP (before the pandemic), while O3 concentration increased by about 40.9% during DP due to a lower concentration of NO2 restraining the decomposition of O3 via the reaction of NO with O3. The number count of carbonaceous particles during DP decreased by 20.2% compared to that during BP due to the sharp reduction of factory production and vehicular transportation during DP. Dust particles during DP exhibited weaker 23Na+, 56Fe+, and 79PO3− signals than those during BP, suggesting that dust particles during DP were mostly derived from mineral dust rather than industrial sources. The total particles during DP peaked at a larger size than those during BP, due to the higher fraction of secondary inorganic ions through the enhanced heterogeneous aqueous oxidation. The unscaled size distribution of total particles peaked at 0.50 µm during BP and at 0.66–0.70 µm during DP, suggesting that particles remained for a long time in the atmosphere and went through a strong aging process during DP. The single particles during DP were more aged than those during BP, owing to the stronger atmospheric oxidizing capacity during DP.
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spelling doaj-art-73954983befb40a2b17f0227ca564a842025-02-09T12:19:28ZengSpringerAerosol and Air Quality Research1680-85842071-14092024-12-012081716172610.4209/aaqr.2020.06.0321Impact of the COVID-19 Event on the Characteristics of Atmospheric Single Particle in the Northern ChinaZheng Li0Jingjing Meng1Ling Zhou2Ruiwen Zhou3Mengxuan Fu4Yachen Wang5Yanan Yi6Aijing Song7Qingchun Guo8Zhanfang Hou9Li Yan10School of Environment and Planning, Liaocheng UniversitySchool of Environment and Planning, Liaocheng UniversityCollege of Resources and Environment, Xingtai UniversitySchool of Environment and Planning, Liaocheng UniversitySchool of Environment and Planning, Liaocheng UniversitySchool of Environment and Planning, Liaocheng UniversitySchool of Environment and Planning, Liaocheng UniversitySchool of Environment and Planning, Liaocheng UniversitySchool of Environment and Planning, Liaocheng UniversitySchool of Environment and Planning, Liaocheng UniversityChinese Academy for Environmental PlanningAbstract The COVID-19 event triggered global attention which broke out at the end of 2019. To investigate the impact of the COVID-19 pandemic prevention and control actions on the chemical composition, size distribution, and mixing state of individual particles, real-time individual particles in the urban atmosphere of the Northern China were analyzed using single particle aerosol mass spectrometry (SPAMS) during January 16 to February 4, 2020. The results showed that the concentrations of PM2.5, NOx, and CO were lower during DP (during the pandemic) than those during BP (before the pandemic), while O3 concentration increased by about 40.9% during DP due to a lower concentration of NO2 restraining the decomposition of O3 via the reaction of NO with O3. The number count of carbonaceous particles during DP decreased by 20.2% compared to that during BP due to the sharp reduction of factory production and vehicular transportation during DP. Dust particles during DP exhibited weaker 23Na+, 56Fe+, and 79PO3− signals than those during BP, suggesting that dust particles during DP were mostly derived from mineral dust rather than industrial sources. The total particles during DP peaked at a larger size than those during BP, due to the higher fraction of secondary inorganic ions through the enhanced heterogeneous aqueous oxidation. The unscaled size distribution of total particles peaked at 0.50 µm during BP and at 0.66–0.70 µm during DP, suggesting that particles remained for a long time in the atmosphere and went through a strong aging process during DP. The single particles during DP were more aged than those during BP, owing to the stronger atmospheric oxidizing capacity during DP.https://doi.org/10.4209/aaqr.2020.06.0321Size distributionMixing stateCOVID-19 pandemicthe North China Plain (NCP)Single particle aerosol mass spectrometry (SPAMS)
spellingShingle Zheng Li
Jingjing Meng
Ling Zhou
Ruiwen Zhou
Mengxuan Fu
Yachen Wang
Yanan Yi
Aijing Song
Qingchun Guo
Zhanfang Hou
Li Yan
Impact of the COVID-19 Event on the Characteristics of Atmospheric Single Particle in the Northern China
Aerosol and Air Quality Research
Size distribution
Mixing state
COVID-19 pandemic
the North China Plain (NCP)
Single particle aerosol mass spectrometry (SPAMS)
title Impact of the COVID-19 Event on the Characteristics of Atmospheric Single Particle in the Northern China
title_full Impact of the COVID-19 Event on the Characteristics of Atmospheric Single Particle in the Northern China
title_fullStr Impact of the COVID-19 Event on the Characteristics of Atmospheric Single Particle in the Northern China
title_full_unstemmed Impact of the COVID-19 Event on the Characteristics of Atmospheric Single Particle in the Northern China
title_short Impact of the COVID-19 Event on the Characteristics of Atmospheric Single Particle in the Northern China
title_sort impact of the covid 19 event on the characteristics of atmospheric single particle in the northern china
topic Size distribution
Mixing state
COVID-19 pandemic
the North China Plain (NCP)
Single particle aerosol mass spectrometry (SPAMS)
url https://doi.org/10.4209/aaqr.2020.06.0321
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