Green hydrothermal approach for the synthesis of carbon quantum dots from waste tea bags for acrylamide detection in drinking water: A fluorescence assay validated by HPLC-PDA analysis

The study focused on converting tea bag waste into strong fluorescence carbon quantum dots (TBW-CQDs) for the detection of acrylamide in drinking water, antimicrobial activity, and photocatalytic degradation. The TBW-CQDs exhibited blue luminescence and maximum absorbance at 287 nm under UV light an...

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Main Authors: Nikhil Sharma, Sweezee Thakur, Aarti Bains, Gulden Goksen, Nemat Ali, Mushtaq Ahmad Ansari, Anna Kopsacheili, Charalampos Proestos, Prince Chawla
Format: Article
Language:English
Published: Elsevier 2025-01-01
Series:Food Chemistry: X
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Online Access:http://www.sciencedirect.com/science/article/pii/S2590157524009313
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author Nikhil Sharma
Sweezee Thakur
Aarti Bains
Gulden Goksen
Nemat Ali
Mushtaq Ahmad Ansari
Anna Kopsacheili
Charalampos Proestos
Prince Chawla
author_facet Nikhil Sharma
Sweezee Thakur
Aarti Bains
Gulden Goksen
Nemat Ali
Mushtaq Ahmad Ansari
Anna Kopsacheili
Charalampos Proestos
Prince Chawla
author_sort Nikhil Sharma
collection DOAJ
description The study focused on converting tea bag waste into strong fluorescence carbon quantum dots (TBW-CQDs) for the detection of acrylamide in drinking water, antimicrobial activity, and photocatalytic degradation. The TBW-CQDs exhibited blue luminescence and maximum absorbance at 287 nm under UV light and distinctive fluorescence emission and excitation wavelengths at 425 nm and 287 nm, respectively. TBW-CQDs revealed a particle size of 8.12 ± 0.06 nm with a spherical morphology followed by an abundance of 59.29 % carbon and 39.82 % oxygen. For acrylamide extraction from water, the QuEChERS method was established, which exhibited a recovery rate of 97 to 99 %. The fluorescence-based sensor exhibited a low limit of detection of 0.35376 ppm, which was validated by HPLC-PDA (LOD 0.300688 ppm). TBW-CQDs degraded 90.62 % of indigo carmine and 93.19 % of methylene blue under bright sunlight. In conclusion, the fabricated TBW-CQDs provide a promising, cost-effective, and precise approach to acrylamide detection in drinking water.
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spelling doaj-art-7efa57fd15b74199a9920db97c5c14982025-02-12T05:31:47ZengElsevierFood Chemistry: X2590-15752025-01-0125102043Green hydrothermal approach for the synthesis of carbon quantum dots from waste tea bags for acrylamide detection in drinking water: A fluorescence assay validated by HPLC-PDA analysisNikhil Sharma0Sweezee Thakur1Aarti Bains2Gulden Goksen3Nemat Ali4Mushtaq Ahmad Ansari5Anna Kopsacheili6Charalampos Proestos7Prince Chawla8Department of Food Technology and Nutrition, School of Agriculture, Lovely Professional University, Phagwara, 144411, IndiaDepartment of Food Technology and Processing, School of Health Sciences, Amity University, Punjab, Mohali 140306, IndiaDepartment of Microbiology, Lovely Professional University, Phagwara 144411, IndiaDepartment of Food Technology, Vocational School of Technical Sciences at Mersin Tarsus Organized Industrial Zone, Tarsus University Mersin, TurkeyDepartment of Pharmacology and Toxicology, College of Pharmacy, King Saud University, P.O.Box 2457, Riyadh 11451, Saudi Arabia.Department of Pharmacology and Toxicology, College of Pharmacy, King Saud University, P.O.Box 2457, Riyadh 11451, Saudi Arabia.Food Chemistry Laboratory, Department of Chemistry, National and Kapodistrian University of Athens, Panepistimiopolis Zographou, 15771 Athens, GreeceFood Chemistry Laboratory, Department of Chemistry, National and Kapodistrian University of Athens, Panepistimiopolis Zographou, 15771 Athens, Greece; Corresponding authors.Department of Food Technology and Nutrition, School of Agriculture, Lovely Professional University, Phagwara, 144411, India; Corresponding authors.The study focused on converting tea bag waste into strong fluorescence carbon quantum dots (TBW-CQDs) for the detection of acrylamide in drinking water, antimicrobial activity, and photocatalytic degradation. The TBW-CQDs exhibited blue luminescence and maximum absorbance at 287 nm under UV light and distinctive fluorescence emission and excitation wavelengths at 425 nm and 287 nm, respectively. TBW-CQDs revealed a particle size of 8.12 ± 0.06 nm with a spherical morphology followed by an abundance of 59.29 % carbon and 39.82 % oxygen. For acrylamide extraction from water, the QuEChERS method was established, which exhibited a recovery rate of 97 to 99 %. The fluorescence-based sensor exhibited a low limit of detection of 0.35376 ppm, which was validated by HPLC-PDA (LOD 0.300688 ppm). TBW-CQDs degraded 90.62 % of indigo carmine and 93.19 % of methylene blue under bright sunlight. In conclusion, the fabricated TBW-CQDs provide a promising, cost-effective, and precise approach to acrylamide detection in drinking water.http://www.sciencedirect.com/science/article/pii/S2590157524009313Tea bagHydrothermalCarbon quantum dotsAcrylamide detectionHPLC
spellingShingle Nikhil Sharma
Sweezee Thakur
Aarti Bains
Gulden Goksen
Nemat Ali
Mushtaq Ahmad Ansari
Anna Kopsacheili
Charalampos Proestos
Prince Chawla
Green hydrothermal approach for the synthesis of carbon quantum dots from waste tea bags for acrylamide detection in drinking water: A fluorescence assay validated by HPLC-PDA analysis
Food Chemistry: X
Tea bag
Hydrothermal
Carbon quantum dots
Acrylamide detection
HPLC
title Green hydrothermal approach for the synthesis of carbon quantum dots from waste tea bags for acrylamide detection in drinking water: A fluorescence assay validated by HPLC-PDA analysis
title_full Green hydrothermal approach for the synthesis of carbon quantum dots from waste tea bags for acrylamide detection in drinking water: A fluorescence assay validated by HPLC-PDA analysis
title_fullStr Green hydrothermal approach for the synthesis of carbon quantum dots from waste tea bags for acrylamide detection in drinking water: A fluorescence assay validated by HPLC-PDA analysis
title_full_unstemmed Green hydrothermal approach for the synthesis of carbon quantum dots from waste tea bags for acrylamide detection in drinking water: A fluorescence assay validated by HPLC-PDA analysis
title_short Green hydrothermal approach for the synthesis of carbon quantum dots from waste tea bags for acrylamide detection in drinking water: A fluorescence assay validated by HPLC-PDA analysis
title_sort green hydrothermal approach for the synthesis of carbon quantum dots from waste tea bags for acrylamide detection in drinking water a fluorescence assay validated by hplc pda analysis
topic Tea bag
Hydrothermal
Carbon quantum dots
Acrylamide detection
HPLC
url http://www.sciencedirect.com/science/article/pii/S2590157524009313
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