Five-year Record of Black Carbon Concentrations in Urban Wanzhou, Sichuan Basin, China

Abstract The atmospheric fine particle black carbon (BC) was measured from June 2013 till February 2018 in Wanzhou District, the second largest metropolitan area in Chongqing Municipality, China, which is located in the eastern Sichuan Basin. The average daily concentration ranged from 0.5 to 10.4 µ...

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Main Authors: Yimin Huang, Liuyi Zhang, Yang Qiu, Yang Chen, Guangming Shi, Tingzhen Li, Lei Zhang, Fumo Yang
Format: Article
Language:English
Published: Springer 2020-04-01
Series:Aerosol and Air Quality Research
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Online Access:https://doi.org/10.4209/aaqr.2019.10.0516
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author Yimin Huang
Liuyi Zhang
Yang Qiu
Yang Chen
Guangming Shi
Tingzhen Li
Lei Zhang
Fumo Yang
author_facet Yimin Huang
Liuyi Zhang
Yang Qiu
Yang Chen
Guangming Shi
Tingzhen Li
Lei Zhang
Fumo Yang
author_sort Yimin Huang
collection DOAJ
description Abstract The atmospheric fine particle black carbon (BC) was measured from June 2013 till February 2018 in Wanzhou District, the second largest metropolitan area in Chongqing Municipality, China, which is located in the eastern Sichuan Basin. The average daily concentration ranged from 0.5 to 10.4 µg m−3, with a mean of 4.4 ± 2.2 µg m−3, and the annual mean displayed a significantly decreasing trend, from 5.3 µg m−3 in 2013 to 3.7 µg m−3 in 2017. The frequency distribution of the average daily concentrations during the years 2014–2017 skewed toward lower values (compared to the rest of the study period), with over 60% falling between 1 and 5 µg m−3. The BC exhibited a seasonal pattern, with the highest concentrations being reported during winter, followed by spring and fall, and the lowest ones during summer, as well as a double-peaked diel variability all year round, with a morning peak occurring between 07:00 and 09:00 and an evening peak between 19:00 and 21:00. Furthermore, the concentration was negatively correlated with the planetary boundary layer (PBL) height and influenced by the strong scavenging effect of precipitation. An inverse relationship between the concentration and the wind speed was observed when the latter was below 2.0 m s−1. The wind direction also affected the concentration, with easterly and southeasterly winds accompanying higher levels of BC regardless of the season.
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issn 1680-8584
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language English
publishDate 2020-04-01
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series Aerosol and Air Quality Research
spelling doaj-art-b5987a9aa19446a0b5d931d75602e1c42025-02-09T12:19:00ZengSpringerAerosol and Air Quality Research1680-85842071-14092020-04-012061282129310.4209/aaqr.2019.10.0516Five-year Record of Black Carbon Concentrations in Urban Wanzhou, Sichuan Basin, ChinaYimin Huang0Liuyi Zhang1Yang Qiu2Yang Chen3Guangming Shi4Tingzhen Li5Lei Zhang6Fumo Yang7Key Laboratory of Water Environment Evolution and Pollution Control in Three Gorges Reservoir, Chongqing Three Gorges UniversityKey Laboratory of Water Environment Evolution and Pollution Control in Three Gorges Reservoir, Chongqing Three Gorges UniversityNational Engineering Research Center for Flue Gas Desulfurization, Department of Environmental Science and Engineering, Sichuan UniversityChongqing Institute of Green and Intelligent Technology, Chinese Academy of SciencesNational Engineering Research Center for Flue Gas Desulfurization, Department of Environmental Science and Engineering, Sichuan UniversityKey Laboratory of Water Environment Evolution and Pollution Control in Three Gorges Reservoir, Chongqing Three Gorges UniversityKey Laboratory of Water Environment Evolution and Pollution Control in Three Gorges Reservoir, Chongqing Three Gorges UniversityKey Laboratory of Water Environment Evolution and Pollution Control in Three Gorges Reservoir, Chongqing Three Gorges UniversityAbstract The atmospheric fine particle black carbon (BC) was measured from June 2013 till February 2018 in Wanzhou District, the second largest metropolitan area in Chongqing Municipality, China, which is located in the eastern Sichuan Basin. The average daily concentration ranged from 0.5 to 10.4 µg m−3, with a mean of 4.4 ± 2.2 µg m−3, and the annual mean displayed a significantly decreasing trend, from 5.3 µg m−3 in 2013 to 3.7 µg m−3 in 2017. The frequency distribution of the average daily concentrations during the years 2014–2017 skewed toward lower values (compared to the rest of the study period), with over 60% falling between 1 and 5 µg m−3. The BC exhibited a seasonal pattern, with the highest concentrations being reported during winter, followed by spring and fall, and the lowest ones during summer, as well as a double-peaked diel variability all year round, with a morning peak occurring between 07:00 and 09:00 and an evening peak between 19:00 and 21:00. Furthermore, the concentration was negatively correlated with the planetary boundary layer (PBL) height and influenced by the strong scavenging effect of precipitation. An inverse relationship between the concentration and the wind speed was observed when the latter was below 2.0 m s−1. The wind direction also affected the concentration, with easterly and southeasterly winds accompanying higher levels of BC regardless of the season.https://doi.org/10.4209/aaqr.2019.10.0516Black carbonSeasonal variationDiel variationMeteorological parameters
spellingShingle Yimin Huang
Liuyi Zhang
Yang Qiu
Yang Chen
Guangming Shi
Tingzhen Li
Lei Zhang
Fumo Yang
Five-year Record of Black Carbon Concentrations in Urban Wanzhou, Sichuan Basin, China
Aerosol and Air Quality Research
Black carbon
Seasonal variation
Diel variation
Meteorological parameters
title Five-year Record of Black Carbon Concentrations in Urban Wanzhou, Sichuan Basin, China
title_full Five-year Record of Black Carbon Concentrations in Urban Wanzhou, Sichuan Basin, China
title_fullStr Five-year Record of Black Carbon Concentrations in Urban Wanzhou, Sichuan Basin, China
title_full_unstemmed Five-year Record of Black Carbon Concentrations in Urban Wanzhou, Sichuan Basin, China
title_short Five-year Record of Black Carbon Concentrations in Urban Wanzhou, Sichuan Basin, China
title_sort five year record of black carbon concentrations in urban wanzhou sichuan basin china
topic Black carbon
Seasonal variation
Diel variation
Meteorological parameters
url https://doi.org/10.4209/aaqr.2019.10.0516
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