Spin-bearing molecules as optically addressable platforms for quantum technologies

Efforts to harness quantum hardware relying on quantum mechanical principles have been steadily progressing. The search for novel material platforms that could spur the progress by providing new functionalities for solving the outstanding technological problems is however still active. Any physical...

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Main Authors: Kuppusamy Senthil Kumar, Hunger David, Ruben Mario, Goldner Philippe, Serrano Diana
Format: Article
Language:English
Published: De Gruyter 2024-10-01
Series:Nanophotonics
Subjects:
Online Access:https://doi.org/10.1515/nanoph-2024-0420
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author Kuppusamy Senthil Kumar
Hunger David
Ruben Mario
Goldner Philippe
Serrano Diana
author_facet Kuppusamy Senthil Kumar
Hunger David
Ruben Mario
Goldner Philippe
Serrano Diana
author_sort Kuppusamy Senthil Kumar
collection DOAJ
description Efforts to harness quantum hardware relying on quantum mechanical principles have been steadily progressing. The search for novel material platforms that could spur the progress by providing new functionalities for solving the outstanding technological problems is however still active. Any physical property presenting two distinct energy states that can be found in a long-lived superposition state can serve as a quantum bit (qubit), the basic information processing unit in quantum technologies. Molecular systems that can feature electron and/or nuclear spin states together with optical transitions are one of the material platforms that can serve as optically addressable qubits. The attractiveness of molecular systems for quantum technologies relies on the fact that molecular structures of atomically defined nature can be obtained in endless diversity of chemical compositions. Crucially, by harnessing the molecular design protocols, the optical and spin (electronic and nuclear) properties of molecules can be tailored, aiding the design of optically addressable spin qubits and quantum sensors. In this contribution, we present a concise and collective discussion of optically addressable spin-bearing molecules – namely, organic molecules, transition metal (TM) and rare-earth ion (REI) complexes – and highlight recent results such as chemical tuning of optical and electron spin quantum coherence, optical spin initialization and readout, intramolecular quantum teleportation, optical coherent storage, and photonic-enhanced optical addressing. We envision that optically addressable spin-carrying molecules could become a scalable building block of quantum hardware for applications in the fields of quantum sensing, quantum communication and quantum computing.
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spelling doaj-art-ee8beb367de14640b6569a237cdcb7ca2025-02-10T13:24:47ZengDe GruyterNanophotonics2192-86142024-10-0113244357437910.1515/nanoph-2024-0420Spin-bearing molecules as optically addressable platforms for quantum technologiesKuppusamy Senthil Kumar0Hunger David1Ruben Mario2Goldner Philippe3Serrano Diana4Institute for Quantum Materials and Technologies (IQMT), Karlsruhe Institute of Technology (KIT), Karlsruhe, GermanyInstitute for Quantum Materials and Technologies (IQMT), Karlsruhe Institute of Technology (KIT), Karlsruhe, GermanyInstitute for Quantum Materials and Technologies (IQMT), Karlsruhe Institute of Technology (KIT), Karlsruhe, GermanyChimie ParisTech, 129667PSL University, CNRS, Institut de Recherche de Chimie Paris, Paris, FranceChimie ParisTech, 129667PSL University, CNRS, Institut de Recherche de Chimie Paris, Paris, FranceEfforts to harness quantum hardware relying on quantum mechanical principles have been steadily progressing. The search for novel material platforms that could spur the progress by providing new functionalities for solving the outstanding technological problems is however still active. Any physical property presenting two distinct energy states that can be found in a long-lived superposition state can serve as a quantum bit (qubit), the basic information processing unit in quantum technologies. Molecular systems that can feature electron and/or nuclear spin states together with optical transitions are one of the material platforms that can serve as optically addressable qubits. The attractiveness of molecular systems for quantum technologies relies on the fact that molecular structures of atomically defined nature can be obtained in endless diversity of chemical compositions. Crucially, by harnessing the molecular design protocols, the optical and spin (electronic and nuclear) properties of molecules can be tailored, aiding the design of optically addressable spin qubits and quantum sensors. In this contribution, we present a concise and collective discussion of optically addressable spin-bearing molecules – namely, organic molecules, transition metal (TM) and rare-earth ion (REI) complexes – and highlight recent results such as chemical tuning of optical and electron spin quantum coherence, optical spin initialization and readout, intramolecular quantum teleportation, optical coherent storage, and photonic-enhanced optical addressing. We envision that optically addressable spin-carrying molecules could become a scalable building block of quantum hardware for applications in the fields of quantum sensing, quantum communication and quantum computing.https://doi.org/10.1515/nanoph-2024-0420organic moleculestransition metal complexesrare-earth ion complexesoptica and spin coherencequbitsquantum technologies
spellingShingle Kuppusamy Senthil Kumar
Hunger David
Ruben Mario
Goldner Philippe
Serrano Diana
Spin-bearing molecules as optically addressable platforms for quantum technologies
Nanophotonics
organic molecules
transition metal complexes
rare-earth ion complexes
optica and spin coherence
qubits
quantum technologies
title Spin-bearing molecules as optically addressable platforms for quantum technologies
title_full Spin-bearing molecules as optically addressable platforms for quantum technologies
title_fullStr Spin-bearing molecules as optically addressable platforms for quantum technologies
title_full_unstemmed Spin-bearing molecules as optically addressable platforms for quantum technologies
title_short Spin-bearing molecules as optically addressable platforms for quantum technologies
title_sort spin bearing molecules as optically addressable platforms for quantum technologies
topic organic molecules
transition metal complexes
rare-earth ion complexes
optica and spin coherence
qubits
quantum technologies
url https://doi.org/10.1515/nanoph-2024-0420
work_keys_str_mv AT kuppusamysenthilkumar spinbearingmoleculesasopticallyaddressableplatformsforquantumtechnologies
AT hungerdavid spinbearingmoleculesasopticallyaddressableplatformsforquantumtechnologies
AT rubenmario spinbearingmoleculesasopticallyaddressableplatformsforquantumtechnologies
AT goldnerphilippe spinbearingmoleculesasopticallyaddressableplatformsforquantumtechnologies
AT serranodiana spinbearingmoleculesasopticallyaddressableplatformsforquantumtechnologies